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Do you mean crossed modules internal to fd Lie algebras? Or something invariant under (weak) equivalence? One could talk of βfinite typeβ Lie algebra crossed modules, for instance ^Ξ©π€βPπ€ is equivalent to the Lβ-algebra iββπ€, and so as an Lβ-algebra it has finite-dimensional homology groups (of the underlying chain complex).
The question of simple-connectedness is a bit more tricky. If you have a Lie algebra crossed module that integrates to a smooth group stack, then one could ask whether the underlying shape of that group stack is simply-connected.
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